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Abstract: (arXiv)
Ultracold polar molecules offer strong electric dipole moments and rich internal structure, which makes them ideal building blocks to explore exotic quantum matter, implement novel quantum information schemes, or test fundamental symmetries of nature. Realizing their full potential requires cooling interacting molecular gases deeply into the quantum degenerate regime. However, the complexity of molecules which makes their collisions intrinsically unstable at the short range, even for nonreactive molecules, has so far prevented the cooling to quantum degeneracy in three dimensions. Here, we demonstrate evaporative cooling of a three-dimensional gas of fermionic sodium-potassium molecules to well below the Fermi temperature using microwave shielding. The molecules are protected from reaching short range with a repulsive barrier engineered by coupling rotational states with a blue-detuned circularly polarized microwave. The microwave dressing induces strong tunable dipolar interactions between the molecules, leading to high elastic collision rates that can exceed the inelastic ones by at least a factor of 460. This large elastic-to-inelastic collision ratio allows us to cool the molecular gas down to 21 nanokelvin, corresponding to 0.36 times the Fermi temperature. Such unprecedentedly cold and dense samples of polar molecules open the path to the exploration of novel many-body phenomena, such as the long-sought topological p-wave superfluid states of ultracold matter.
Note:
  • 11 pages, 7 figures
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    Stable topological superfluid phase of ultracold polar fermionic molecules
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    • G.V. Shlyapnikov
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    Wu, Z
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    • L. Lassablière
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    • T. Langen
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    Quantum phases of a twodimensional dipolar fermi gas
    • G.M. Bruun
      ,
    • E. Taylor
      • Phys.Rev.Lett. 101 (2008) 245301
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    Liquid and crystal phases of dipolar fermions in two dimensions
    • N. Matveeva
      ,
    • S. Giorgini
      • Phys.Rev.Lett. 109 (2012) 200401
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    Condensed matter theory of dipolar quantum gases
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    • P. Zoller
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    & Cˆ oté, R. Schemes
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    Ni, K.-K
    • T. Rosenband
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    • D.D. Grimes
      • Science 9 (2018) 6830-6838
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    Scattering of ultracold molecules in the highly resonant regime
    • M. Mayle
      ,
    • G. Quéméner
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    • B.P. Ruzic
      ,
    • J.L. Bohn
      • Phys.Rev.A 87 (2013) 012709
  • [14]
    Photoinduced two-body loss of ultracold molecules
    • A. Christianen
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    • M.W. Zwierlein
      ,
    • G.C. Groenenboom
      ,
    • T. Karman
      • Phys.Rev.Lett. 123 (2019) 123402
  • [15]
    Loss of ultracold 87 Rb133 Cs molecules via optical excitation of long-lived two-body collision complexes
    • P.D. Gregory
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    • J.A. Blackmore
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    • S.L. Bromley
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    • S.L. Cornish
      • Phys.Rev.Lett. 124 (2020) 163402
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    Photo-excitation of long-lived transient intermediates in ultracold reactions
    • Y. Liu
      • Nature Phys. 16 (2020) 1132-1136
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    Collisions of ultracold molecules in bright and dark optical dipole traps
    • R. Bause
      • Phys.Rev.Res. 3 (2021) 033013
  • [18]
    Probing photoinduced two-body loss of ultracold nonreactive bosonic 23 Na87 Rb and 23 Na39 K molecules
    • P. Gersema
      • Phys.Rev.Lett. 127 (2021) 163401
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    & Ye, J. Cold
    • J.L. Bohn
      ,
    • A.M. Rey
      • Science 357 (2017) 1002-1010
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    Creation of a low-entropy quantum gas of polar molecules in an optical lattice
    • S.A. Moses
      • Science 350 (2015) 659-662
  • [22]
    A degenerate Fermi gas of polar molecules
    • L. De Marco
      • Science 363 (2019) 853-856
  • [23]
    Transition from a polaronic condensate to a degenerate Fermi gas of heteronuclear molecules. Preprint at
    • M. Duda
  • [24]
    Dipolar collisions of polar molecules in the quantum regime
    • K.-K. Ni
      • Nature 464 (2010) 1324-1328
  • [25]
    ˙
    • P.S. Zuchowski
      ,
    • J.M. Hutson
      • Phys.Rev.A 81 (2010) 060703