Direct measurement of the 3^{3}He+^{+} magnetic moments

Jun 8, 2022
6 pages
Published in:
  • Nature 606 (2022) 7916, 878-883,
  • Nature (2022)
  • Published: Jun 8, 2022
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Abstract: (Springer)
Helium-3 has nowadays become one of the most important candidates for studies in fundamental physics13^{1–3}, nuclear and atomic structure4,5^{4,5}, magnetometry and metrology6^{6}, as well as chemistry and medicine7,8^{7,8}. In particular, 3^{3}He nuclear magnetic resonance (NMR) probes have been proposed as a new standard for absolute magnetometry6,9^{6,9}. This requires a high-accuracy value for the 3^{3}He nuclear magnetic moment, which, however, has so far been determined only indirectly and with a relative precision of 12 parts per billon10,11^{10,11}. Here we investigate the 3^{3}He+^{+} ground-state hyperfine structure in a Penning trap to directly measure the nuclear g-factor of 3^{3}He+gI=4.2550996069(30)stat(17)sys^{+}{g}_{I}^{{\prime} }=-\,4.2550996069(30{)}_{{\rm{stat}}}(17{)}_{{\rm{sys}}}, the zero-field hyperfine splitting EHFSexp=8,665,649,865.77(26)stat(1)sys{E}_{{\rm{HFS}}}^{\exp }=-\,8,\,665,\,649,\,865.77{(26)}_{{\rm{stat}}}{(1)}_{{\rm{sys}}} Hz and the bound electron g-factor geexp=2.00217741579(34)stat(30)sys{g}_{e}^{{\rm{\exp }}}=-\,2.00217741579(34{)}_{{\rm{stat}}}(30{)}_{{\rm{sys}}}. The latter is consistent with our theoretical value getheo=2.00217741625223(39){g}_{e}^{{\rm{theo}}}=-\,2.00217741625223(39) based on parameters and fundamental constants from ref. 12^{12}. Our measured value for the 3^{3}He+^{+} nuclear g-factor enables determination of the g-factor of the bare nucleus gI=4.2552506997(30)stat(17)sys(1)theo{g}_{I}=-\,4.2552506997(30{)}_{{\rm{stat}}}(17{)}_{{\rm{sys}}}(1{)}_{{\rm{theo}}} via our accurate calculation of the diamagnetic shielding constant13σ3He+=0.00003550738(3)^{13}{\sigma }_{{}^{3}{\mathrm{He}}^{+}}=0.00003550738(3). This constitutes a direct calibration for 3^{3}He NMR probes and an improvement of the precision by one order of magnitude compared to previous indirect results. The measured zero-field hyperfine splitting improves the precision by two orders of magnitude compared to the previous most precise value14^{14} and enables us to determine the Zemach radius15^{15} to rZ=2.608(24){r}_{Z}=2.608(24) fm.