Observation of the Magnonic Dicke Superradiant Phase Transition

Jan 3, 2024
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202220232024017
Abstract: (arXiv)
Two-level atoms coupled with single-mode cavity photons are predicted to exhibit a quantum phase transition when the coupling strength exceeds a critical value, entering a phase in which atomic polarization and photonic field are finite even at zero temperature and without external driving. However, this phenomenon, the superradiant phase transition (SRPT), is forbidden by a no-go theorem due to the existence of the diamagnetic term in the Hamiltonian. Here, we present spectroscopic evidence for a magnonic SRPT in ErFeO3_3, where the role of the photonic mode (two-level atoms) in the photonic SRPT is played by an Fe3+^{3+} magnon mode (Er3+^{3+} spins). The absence of the diamagnetic term in the Fe3+^{3+}-Er3+^{3+} exchange coupling ensures that the no-go theorem does not apply. Terahertz and gigahertz magnetospectroscopy experiments revealed the signatures of the SRPT -- a kink and a softening, respectively, of two spin-magnon hybridized modes at the critical point.