Stability of β\beta″ nano-phases in Al-Mg-Si(-Cu) alloy under high dose ion irradiation

2017
13 pages
Published in:
  • Acta Mater. 128 (2017) 64-76

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Abstract: (Elsevier)
The microstructure of a 6061-T6 Al alloy subjected to ion irradiation at 95 and 165 displacements per atom (dpa) has been evaluated by transmission electron microscopy and atom-probe tomography. The initial microstructure of the alloy is dominated by needle-shaped β″ precipitates. After 95 dpa irradiation, the β″ precipitates display a slight lattice distortion and are partially dissolved, together with the formation of a new phase. After 165 dpa irradiation, the β″ precipitates are completely dissolved, the new phase has grown and a high density of clusters rich in Mg, Si, Cu and Cr is observed. The determination of ballistic versus radiation enhanced diffusion coefficients shows that enhanced diffusion is predominant for β” dissolution. The formation and growth of the new particles may be caused by radiation induced segregation. Solute drag by vacancies or mixed dumbbell interstitials migration could explain the diffusion of some elements as Si or Cr towards the new particles.
  • [1]
    Jules Horowitz Reactor: a high performance material testing reactor
    • D. Iracane
      ,
    • P. Chaix
      ,
    • A. Alamo
      • Comptes Rendus Physique 9 (2008) 445-456
  • [2]
    The crystal structure of the b00 phase in AleMgeSi alloys
    • S.J. Andersen
      ,
    • H.W. Zandbergen
      ,
    • J. Jansen
      ,
    • C. TrÆholt
      ,
    • U. Tundal
    et al.
      • Acta Mater. 46 (1998) 3283-3298
  • [3]
    The crystal structure of the b0 phase in AleMgeSi alloys
    • R. Vissers
      ,
    • M.A. van Huis
      ,
    • J. Jansen
      ,
    • H.W. Zandbergen
      ,
    • C.D. Marioara
    et al.
      • Acta Mater. 55 (2007) 3815-3823
  • [4]
    The structural relation between precipitates in AleMgeSi alloys, the Al-matrix and diamond silicon, with emphasis on the trigonal phase U1-MgAl2Si2
    • S.J. Andersen
      ,
    • C.D. Marioara
      ,
    • R. Vissers
      ,
    • A. Frøseth
      ,
    • H.W. Zandbergen
      • Mater.Sci.Eng.A 444 (2007) 157-169
  • [5]
    Crystal structure of the orthorhombic U2-Al4Mg4Si4 precipitate in the AleMgeSi alloy system and its relation to the b0 and b00 phases
    • S.J. Andersen
      ,
    • C.D. Marioara
      ,
    • A. Frøseth
      ,
    • R. Vissers
      ,
    • H.W. Zandbergen
      • Mater.Sci.Eng.A 390 (2005) 127-138
  • [6]
    In situ characterization of b0 0 precipitation in an AleMgeSi alloy by anisotropic small-angle neutron scattering on a single crystal
    • C.S.T. Chang
      ,
    • F. De Geuser
      ,
    • J. Banhart
      • J. Appl Crystallogr. 48 (2015) 455-463
  • [7]
    Structure determination of Mg5Si6 particles in Al by dynamic electron diffraction studies
    • H.W. Zandbergen
      ,
    • S.J. Andersen
      ,
    • J. Jansen
      • Science 277 (1997) 1221-1225
  • [8]
    The precipitation sequence in AleMgeSi alloys
    • G.A. Edwards
      ,
    • K. Stiller
      ,
    • G.L. Dunlop
      ,
    • M.J. Couper
      • Acta Mater. 46 (1998) 3893-3904
  • [9]
    Crystal structure of the b0 0 phase in an Alel.0mass%Mg2Sie0.4mass%Si alloy
    • K. Matsuda
      ,
    • T. Naoi
      ,
    • K. Fujii
      ,
    • Y. Uetani
      ,
    • T. Sato
    et al.
      • Mater.Sci.Eng.A 262 (1999) 232-237
  • [10]
    A first-principles study of the b’’-phase in Al-Mg-Si alloys
    • P.M. Derlet
      ,
    • S.J. Andersen
      ,
    • C.D. Marioara
      ,
    • A. Frøseth
      • J.Phys.Condens.Matter 14 (2012) 4011-4024
  • [11]
    Pre-precipitate clusters and precipitation processes in AleMgeSi alloys
    • M. Murayama
      ,
    • K. Hono
      • Acta Mater. 47 (1999) 1537-1548
  • [12]
    Effect of silicon addition on the composition and structure of fine-scale precipitates in Al-Mg-Si alloys
    • N. Maruyama
      ,
    • R. Uemori
      ,
    • N. Hashimoto
      ,
    • M. Saga
      ,
    • M. Kikuchi
      • Scripta Mater. 36 (1997) 89-93
  • [13]
    Comparative study of the b00-phase in a 6xxx Al alloy by 3DAP and HRTEM
    • H.K. Hasting
      ,
    • W. Lefebvre
      ,
    • C. Marioara
      ,
    • J.C. Walmsley
      ,
    • S. Andersen
    et al.
      • Surf.Interface Anal. 39 (2007) 189-194
  • [14]
    Composition of b00 precipitates in AleMgeSi alloys by atom probe tomography and first principles calculations
    • H.S. Hasting
      ,
    • A.G. Frøseth
      ,
    • S.J. Andersen
      ,
    • R. Vissers
      ,
    • J.C. Walmsley
    et al.
      • J.Appl.Phys. 106 (2009) 1235271-1235279
  • [15]
    Detailed atomistic insight into the b00 phase in AleMgeSi alloys
    • P.H. Ninive
      ,
    • A. Strandlie
      ,
    • S. Gulbrandsen-Dahl
      ,
    • W. Lefebvre
      ,
    • C.D. Marioara
    et al.
      • Acta Mater. 69 (2014) 126-134
  • [16]
    The effect of Cu on precipitation in AleMgeSi alloys
    • C.D. Marioara
      ,
    • S.J. Andersen
      ,
    • T.N. Stene
      ,
    • H. Hasting
      ,
    • J. Walmsley
    et al.
      • Phil.Mag. 87 (2007) 3385-3413
  • [17]
    The natural aging and precipitation hardening behaviour of Al-Mg-Si-Cu alloys with different Mg/Si ratios and Cu additions
    • L. Ding
      ,
    • Z. Jia
      ,
    • Z. Zhang
      ,
    • R.E. Sanders
      ,
    • Q. Liu
    et al.
      • Mater.Sci.Eng.A 627 (2015) 119-126
  • [18]
    Atomistic structure of Cu-containing b00 precipitates in an AleMgeSieCu alloy
    • K. Li
      ,
    • A. Beche
      ,
    • M. Song
      ,
    • G. Sha
      ,
    • X. Lu
    et al.
      • Scripta Mater. 75 (2014) 86-89
  • [19]
    HRTEM study of the effect of deformation on the early precipitation behavior in an AA6060 Al-Mg-Si alloy
    • K. Teichmann
      ,
    • C.D. Marioara
      ,
    • S.J. Andersen
      ,
    • K.O. Pedersen
      ,
    • S. Gulbrandsen-Dahl
    et al.
      • Phil.Mag. 91 (2011) 3744-3754
  • [20]
    Study of intergrown L and Q’ precipitates in Al-Mg-Si-Cu alloys
    • M. Torsӕter
      ,
    • W. Lefebvre
      ,
    • C.D. Marioara
      ,
    • S.J. Andersen
      ,
    • J.C. Walmsley
    et al.
      • Scripta Mater. 64 (2011) 817-820
  • [21]
    4th Int Conf Al Alloys Their Phys. Mech. Prop. Trans Tech Publ. Suisse, 636-643
    • L. Sagalowicz
      ,
    • G. Hug
      ,
    • D. Bechet
      ,
    • P. Sainfort
      ,
    • G. Lapasset
  • [22]
    Phase relations and precipitation in AleMgeSi alloys with Cu additions
    • D.J. Chakrabarti
      ,
    • D.E. Laughlin
      • Prog.Mater.Sci. 49 (2004) 389-410
  • [23]
    Applying precipitate-host lattice coherency for compositional determination of precipitates in Al-Mg-Si-Cu alloys
    • M. Torsӕter
      ,
    • F.J.H. Ehlers
      ,
    • C.D. Marioara
      ,
    • S.J. Andersen
      ,
    • R. Holmestad
      • Phil.Mag. 92 (2012) 3833-3856
  • [24]
    Study of microstructural evolutions of the 6061-T6 aluminium alloy under irradiation (Ph.D. thesis)
    • C. Flament
  • [25]
    Post-b00 phases and their influence on microstructure and hardness in 6xxx Al-Mg-Si alloys, J
    • C.D. Marioara
      ,
    • H. Nordmark
      ,
    • S.J. Andersen
      ,
    • R. Holmestad
      • Mater.Sci. 41 (2006) 471-478